Abstract

Cooking fumes are an important source of volatile organic compounds (VOCs), particulate matter (PM), and carbonyl compounds. The additive is wildly applied in grilling meat for flavor improvement. However, the effects of additives on cooking fumes emissions, such as volatile organic compounds (VOCs), particulate matter (PM), and carbonyl compounds, in meat grilling have not been studied. The impact of four additives, including white pepper, salt, garlic powder, and compound marinade, on the emission characteristics of cooking fumes from the grilling meat was investigated. The concentrations of VOCs and carbonyl compounds in the cooking fumes were analyzed by TD-GC/MS and HPLC, respectively. The PM emission characteristics (mass concentration and size distribution) were measured by DustTrak DRX aerosol monitor in real-time. Results showed that the application of white pepper, salt, garlic powder, and mixed spices could significantly reduce the total particles mass concentration (TPM) emissions during meat-grilling by 65.07%, 47.86%, 32.87%, and 56.01%, respectively. The mass concentration of PM during meat-grilling reached maximum values ranging from 350 to 390 s and gradually fell at the final stages of grilling. The total concentration of 22 representative VOCs emitted from the grilling was significantly increased in grilling meat marinated with compound additives. Aromatic hydrocarbons were the predominant VOCs species, followed by ketone compounds. During the grilling process, formaldehyde, acetaldehyde, propionaldehyde, and acetone were major carbonyl compounds. The low molecular weight carbonyl compounds (C1–C3) in cooking fumes were dominant carbonyl compounds.

Highlights

  • The cooking fumes emitted from cooking activities result in human exposure to particulate matter (PM) and volatile organic compounds (VOCs) [1]

  • The results indicated that all marinade-treatment with white pepper powder, salt, garlic powder, and mixed spices (MS) can reduce the concentration of PM emissions compared to the control testing

  • The meat without any additive marinade generated higher (p < 0.05) total particles mass concentration (TPM) mass concentration compared to the marinated meat with white pepper, salt, garlic powder, and MS during meat-grilling

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Summary

Introduction

The cooking fumes emitted from cooking activities result in human exposure to particulate matter (PM) and volatile organic compounds (VOCs) [1]. The VOCs species are a complex mixture of hazardous chemicals, which consists of benzene series, alkanes, chlorinated VOCs, oxygenated VOCs, and alkenes, and carbonyl compounds [2]. Several studies have proved that PM and VOCs emitted from cooking activities consist of multiple hazardous chemical compounds which are deposited in the alveoli and can cause cardiovascular and respiratory disease or even death. Apart from these negative effects, cooking ultrafine particles can impact human brain activity [4–9]. Characterizing VOCs, PM, and its chemical constituent and exploring beneficial methods for reducing the emission of cooking fumes are significant in improving the healthy environment of food processing or cooking for human beings

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