Abstract

The typical photodetectors can only detect one specific optical spectral band, such as InGaAs and graphene-PbS quantum dots for near-infrared (NIR) light detection, CdS and Si for visible light detection, and ZnO and III-nitrides for UV light detection. So far, none of the developed photodetector can achieve the multicolor detection with arbitrary spectral selectivity, high sensitivity, high speed, high signal-to-noise ratio, high stability, and simplicity (called 6S requirements). Here, we propose a universal strategy to develop multicolor photodetectors with arbitrary spectral selectivity by integrating various semiconductor nanostructures on a wide-bandgap semiconductor or an insulator substrate. Because the photoresponse of each spectral band is determined by each semiconductor nanostructure or the semiconductor substrate, multicolor detection satisfying 6S requirements can be readily satisfied by selecting the right semiconductors.

Highlights

  • The typical photodetectors can only detect one specific optical spectral band, such as InGaAs and graphene-PbS quantum dots for near-infrared (NIR) light detection, CdS and Si for visible light detection, and ZnO and III-nitrides for UV light detection

  • Because the photoresponse of each spectral band is determined by each semiconductor nanostructure or the semiconductor substrate, multicolor detection satisfying 6S requirements can be readily satisfied by selecting the right semiconductors

  • We report a universal strategy for multicolor photodetection with arbitrary spectral selectivity by integrating various semiconductor nanostructures on a wide-bandgap semiconductor or an insulator substrate

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Summary

OPTICS AND PHOTONICS MATERIALS SCIENCE ENGINEERING

Correspondence and requests for materials should be addressed to J.Q.H. (hu.junqing@ dhu.edu.cn) or M.Y.L. None of the developed photodetector can achieve the multicolor detection with arbitrary spectral selectivity, high sensitivity, high speed, high signal-to-noise ratio, high stability, and simplicity (called 6S requirements). We propose a universal strategy to develop multicolor photodetectors with arbitrary spectral selectivity by integrating various semiconductor nanostructures on a wide-bandgap semiconductor or an insulator substrate. One conventional approach is to utilize multiple stacks of optically absorbing materials in a thinfilm structure, such as a quantum-well photodetector using interband/intraband transitions or homo-/heterojunction structures[12,13,14] This stacking approach relies on the quality of the interface between each absorption layer, which makes fabrication difficult and complex, especially for large lattice-mismatched heterojunctions. We report a universal strategy for multicolor photodetection with arbitrary spectral selectivity by integrating various semiconductor nanostructures on a wide-bandgap semiconductor or an insulator substrate. By properly selecting the semiconductors with different bandgaps and high crystal quality, multicolor detection can be achieved with satisfying the 6S requirements

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