Abstract

Metal halide perovskite (MHP) materials are now investigated as the active layer of semiconductor devices such as solar cells and light-emitting diodes (LEDs). Perovskite LEDs (PeLEDs) with high-quality made by a cost-effective process are needed to achieve a commercialized PeLED. To reach this goal, modifying and surface engineering the perovskite emissive thin films can be helpful. The manufacturing process must be economical and time-saving for fabricating an effective commercial device. This work presents an effective postprocessing method to recrystallize the perovskite emissive layer. The method includes both annealing and plasma treatment, which takes a short time and does not need vacuum tools. Applying this process results in a reduction of the MAPbBr3 grain size. It also increases perovskite emitters' carrier recombination rate and photoluminescence quantum yields (PLQY). These results indeed can increase luminance (∼68500 cd/m2), External quantum efficiency (EQE, ∼20.5%), and lifetime (∼350 min).

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