Abstract
The NO/NO2/O3 reaction mechanism of the standard VDI 3783 Part 19 was coupled to the Lagrangian particle model LASAT and quasi-stationary, individual plumes were calculated for a point source under various conditions. First-order conversion rates between NO and NO2 were derived by fitting to these plumes and further simplified to sets of categorized conversion rates which depend on background NO2 concentration, atmospheric stability and time of the day. The rates were applied in the standard airport dispersion model system LASPORT and compared to measured NO2 concentrations at Los Angeles International Airport. The agreement between modelled and measured NO2 concentrations (weekly averages) and ratios NO2 over NOx at monitor stations dominated by airport emissions was in most cases better than a factor of 2 with a Pearson correlation coefficient of about 0.9 or above.
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