Abstract
The synthesis of 2,5-syn disubstituted pyrrolidines from N-SES protected aziridines is described. The key step in the methodology is a 5-endo-trig cyclisation. Application of this reaction in the synthesis of (+)-preussin is reported.
Highlights
The pyrrolidine ring system has been identified as an important pharmacophore in many natural products and drug candidates.[1]
Representative examples of compounds isolated from nature containing a pyrrolidine ring are the antifungal agent (+)-preussin, 1,2 and the pheromone (+)monomorine I, 2.3
We have been evaluating the use of the 5-endo-trig cyclisation[5] for the formation of 2,5-syn disubstituted pyrrolidines.[6,7]
Summary
The pyrrolidine ring system has been identified as an important pharmacophore in many natural products and drug candidates.[1].
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