Abstract
Abstract Magnetic susceptibility was studied on a Ni(II) cyclam complex with iodide, which exhibited an anomalous temperature variation. A diamagnetic spin state at room temperature made a transition into a paramagnetic state below ca. 50 K, and the magnetic susceptibility increased continuously toward a liquid helium temperature. An ESR observation was in good agreement with this magnetic behavior. This finding is unusual in spin crossover phenomena in transition metal ions.
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