Abstract

Understanding superconductivity requires detailed knowledge of the normal electronic state from which it emerges. A nematic electronic state that breaks the rotational symmetry of the lattice can potentially promote unique scattering relevant for superconductivity. Here, we investigate the normal transport of superconducting FeSe$_{1-x}$S$_x$ across a nematic phase transition using high magnetic fields up to 69 T to establish the temperature and field-dependencies. We find that the nematic state is an anomalous non-Fermi liquid, dominated by a linear resistivity at low temperatures that can transform into a Fermi liquid, depending on the composition $x$ and the impurity level. Near the nematic end point, we find an extended temperature regime with $T^{1.5}$ resistivity. The transverse magnetoresistance inside the nematic phase has as a $H^{1.55}$ dependence over a large magnetic field range and it displays an unusual peak at low temperatures inside the nematic phase. Our study reveals anomalous transport inside the nematic phase, driven by the subtle interplay between the changes in the electronic structure of a multi-band system and the unusual scattering processes affected by large magnetic fields and disorder

Highlights

  • Magnetic field is a unique tuning parameter that can suppress superconductivity to reveal the normal low-temperature electronic behavior of many unconventional superconductors [1,2]

  • We find that the nematic state is dominated by a linear resistivity at low temperatures that evolves towards Fermi-liquid behavior, depending on the composition x and the impurity level

  • Near the nematic end point, we find an extended temperature regime with ∼T 1.5 resistivity, different from the behavior found near an antiferromagnetic critical point

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Summary

Methods

Single crystals of FeSe1−xSx were grown by the KCl/AlCl3 chemical vapor transport method [23]. The composition for samples from the same batch was checked using energy-dispersive x-ray (EDX) spectroscopy, as reported previously in Ref. In-plane transport measurements [I||(ab)] were performed in a variable-temperature cryostat in dc fields up to 38 T at HFML, Nijmegen and up to 70 T at LNCMI, Toulouse, with the magnetic field applied mainly along the c axis (transverse magnetoresistance) and in the (ab) conducting plane (longitudinal magnetoresistance) at constant temperatures. The resistivity ρxx and Hall ρxy components were measured using a low-frequency five-probe technique (between 15 and 30 Hz to avoid crosstalk between samples) and were separated by (anti)symmetrizing data measured in positive and negative magnetic fields. Magnetic fields along the c axis suppress superconductivity in fields higher than 20 T for all x values [3]

Results and discussion
Nematic B
Nematic T *
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