Abstract

xwt%Ba0.6Sr0.4TiO3-(1−x)wt%[0.4La (Mg0.5Ti0.5)O3-0.6(La0.5Na0.5)TiO3] (x=0.30, 0.40, 0.50, 0.60, 0.70, 0.80, 0.90, 0.95) ceramics were prepared via a traditional solid-state reaction route. Interesting anomalous dielectric nonlinearity (ADN)—permittivity increased with dc bias electric field (E-field), and low-temperature dielectric relaxation (LTDR) behaviors—were observed within a x range of 0.30∼0.70 for the first time. Based on our experimental facts, it was suggested that the LTDR was originated from a charge-associated process between electron-oxygen vacancy pairs during a thermal stimulation, while the ADN was related with a metastable state of polarized nano-regions (PNRs).

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