Abstract

We present an extensive overview of the phase diagram, spin-wave excitations, and finite-temperature transitions of the anisotropic-exchange magnets on an ideal nearest-neighbor triangular lattice. We investigate transitions between five principal classical phases of the corresponding model: ferromagnetic, N\'{e}el, its dual, and the two stripe phases. Transitions are identified by the spin-wave instabilities and by the Luttinger-Tisza approach. Some of the transitions are direct and others occur via intermediate phases with more complicated forms of ordering. In a portion of the N\'{e}el phase, we find spin-wave instabilities to a long-range spiral-like state. In the stripe phases, quantum fluctuations are mostly negligible, leaving the ordered moment nearly saturated even for the $S=1/2$ case. However, for a two-dimensional surface of the full 3D parameter space, the spin-wave spectrum in one of the stripe phases exhibits an enigmatic accidental degeneracy manifested by pseudo-Goldstone modes. As a result, despite the nearly classical ground state, the ordering transition temperature in a wide region of the phase diagram is significantly suppressed from the mean-field expectation. We identify this accidental degeneracy as due to an exact correspondence to an extended Kitaev-Heisenberg model with emergent symmetries that naturally lead to the pseudo-Goldstone modes. There are previously studied dualities within the Kitaev-Heisenberg model on the triangular lattice that are exposed here in a wider parameter space. One important implication of this correspondence for the $S=1/2$ case is the existence of a region of the spin-liquid phase that is dual to the spin-liquid phase discovered recently by us. We complement our studies by the density-matrix renormalization group of the $S=1/2$ model to confirm some of the duality relations and to verify the existence of the dual spin-liquid phase.

Highlights

  • Ever since the seminal works by Wannier [1] and Anderson [2], a motif of spins on a triangular-lattice network epitomizes the idea of geometric frustration that can give rise to nonmagnetic spin-liquid states [3,4]

  • In real materials desired terms occur along with the other diagonal and offdiagonal components of the anisotropic-exchange matrix that are allowed by the lattice symmetry [12,13,14,15,16]. These terms have proven to be detrimental to the Kitaev spin liquid and so far have prevented its definite realization [12]

  • In our more recent work, Ref. [39], we provided a detailed exploration of the phase diagram of the most generic nearest-neighbor triangular-lattice model in order to find out whether anisotropic-exchange interactions on this lattice can potentially create much desired exotic states

Read more

Summary

INTRODUCTION

Ever since the seminal works by Wannier [1] and Anderson [2], a motif of spins on a triangular-lattice network epitomizes the idea of geometric frustration that can give rise to nonmagnetic spin-liquid states [3,4]. We provide a quasiclassical description of the five principal magnetically ordered single-Q phases that span the 3D phase diagram of the nearest-neighbor anisotropic-exchange model on the triangular lattice These phases are ferromagnetic, 120° Neel, dual 120°, and two different stripe states. While the system is almost classical, large values of the factor f 1⁄4 TMF=TN, which is used to identify a proximity to a quantum-disordered state [23,35], can be highly misleading, questioning it as a useful measure in such cases This surface of accidental degeneracy in the anisotropic-exchange model is identified as corresponding to an extended Kitaev-Heisenberg model.

MODEL AND CLASSICAL PHASES
Classical phase diagram
MAGNON SPECTRA
Stripe-x phase
Stripe-yz phase
Ferromagnetic phase
INSTABILITIES OF MAGNON SPECTRA
Stripe phases
Quantum fluctuations
Thermal fluctuations
CUBIC AXES AND GENERALIZED KITAEV-HEISENBERG MODEL
QUANTUM REALM
Dual spin-liquid region
VIII. SUMMARY
Full Text
Published version (Free)

Talk to us

Join us for a 30 min session where you can share your feedback and ask us any queries you have

Schedule a call