Anisotropic nonlinear Kerr media: Z-scan characterization and interaction with hybridly polarized beams.

Abstract

The interaction of intense laser with matter gives rise to a variety of novel nonlinear optical effects, reflects the nonlinear optical property of a material, and modulates the light propagation behavior. Herein, we investigate anisotropic Kerr nonlinearities induced by both scalar and vectorial optical fields. Firstly, we present the anisotropic third-order nonlinear refraction indexes related to left-hand and right-hand components, which depend on the ellipticity, the dichroism coefficient, the anisotropy coefficient, as well as the crystal orientation angle. Secondly, we develop the elliptically polarized light Z-scan technique for characterizing third-order nonlinear susceptibility tensor in anisotropic nonlinear Kerr media, which is demonstrated experimentally. Lastly, with the known nonlinear optical parameters, we numerically study both the vectorial self-diffraction behaviors and spin angular momentum (SAM) characteristics of hybridly polarized beams induced by an anisotropic Kerr nonlinearity. It is shown that the anisotropic Kerr nonlinearity offers a new approach to manipulate the polarization-structured light field, which has potential applications in SAM manipulation, three-dimensional crystal orientation, and polarization-sensitive detection and sensing.