Abstract
A generalized approach is derived for the analysis of angle-resolved coherent optical wave mixing. Remarkably with this, a signal is calculated to remain efficiently generated for the arbitrary evolution of a quantum superposition state and for energy transfer spanning an ultrawide bandwidth in solution. This approach is compact and applies across matter processes and wave-mixing schemes. A high sensitivity and sampling rate are shown to be intrinsic to angle-resolved wave mixing and an angle-resolved six-wave mixing scheme is proposed for the mapping of molecular structure.
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Schedule a callMore From: Physical review. A, Atomic, molecular, and optical physics
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