Abstract

Cellulose nanocrystals, as well as hydroxypropyl cellulose, can form lyotropic liquid crystals, which can be processed into pigments or glitter products for sustainable coloration. Some stimuli-responsive polymers or nanoparticles are expected to form colorimetric sensors via co-assembly with these cellulosic photonic crystals. The co-assembly behavior of CNCs with polymers is determined by the hydrogen bonds and physical adsorption. Thus, adjusting the molecular chain structure, hydrophilicity, and electrostatic interaction of co-assembled polymers can lead to flexible and tunable colorimetric cellulosic sensors. Despite the advantages of cellulose-based amorphous photonic crystal (APC) pigments or glitters as sustainable and visually captivating sensors, there are still problems in efficient preparation and co-assembly conditions. This editorial will provide a brief discussion of the benefits, applications, and challenges of cellulose-based APCs.

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