Abstract

Analytical expressions are presented that allow the calculation of coherent anti-Stokes Raman spectra (CARS) of gas phase molecules with nonoverlapping lines. The results of the evaluation of Kataoka-Teets and Yuratich convolution integrals are given for six cases: scanning and multiplex CARS where the pump and Stokes laser intensity spectral profiles are Gaussian, Lorentzian, and the mixed configuration of Lorentzian pump and Gaussian Stokes profiles. Useful approximations to these expressions are discussed.

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