Abstract
A study has been made of the available information concerning the variation of the viscosities of acetonitrile—water mixtures with composition in the acetonitrile-rich region. The study shows that the viscosity maximum reported at X(ACN)⋍0.9 is an artifact of an overparameterised curve fitting procedure. The use of a segmented composition model led to some tentative conclusions about the patterns of molecular aggregation of this system.
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