Abstract

Abstract. The Canadian Arctic (> 60∘ N, 60–141∘ W) may undergo drastic changes if the Arctic warming trend continues. For methane (CH4), Arctic reservoirs are large and widespread, and the climate feedbacks from such changes may be potentially substantial. Current bottom-up and top-down estimates of the regional CH4 flux range widely. This study analyzes the recent observations of atmospheric CH4 from five arctic monitoring sites and presents estimates of the regional CH4 fluxes for 2012–2015. The observational data reveal sizeable synoptic summertime enhancements in the atmospheric CH4 that are distinguishable from background variations, which indicate strong regional fluxes (primarily wetland and biomass burning CH4 emissions) around Behchoko and Inuvik in the western Canadian Arctic. Three regional Bayesian inversion modelling systems with two Lagrangian particle dispersion models and three meteorological datasets are applied to estimate fluxes for the Canadian Arctic and show relatively robust results in amplitude and temporal variations across different transport models, prior fluxes, and subregion masking. The estimated mean total CH4 flux for the entire Canadian Arctic is 1.8±0.6 Tg CH4 yr−1. The flux estimate is partitioned into biomass burning of 0.3±0.1 Tg CH4 yr−1 and the remaining natural (wetland) flux of 1.5±0.5 Tg CH4 yr−1. The summer natural CH4 flux estimates clearly show inter-annual variability that is positively correlated with surface temperature anomalies. The results indicate that years with warmer summer conditions result in more wetland CH4 emissions. More data and analysis are required to statistically characterize the dependence of regional CH4 fluxes on the climate in the Arctic. These Arctic measurement sites will aid in quantifying the inter-annual variations and long-term trends in CH4 emissions in the Canadian Arctic.

Highlights

  • Atmospheric methane (CH4) is one of the principal greenhouse gases with a global warming potential (GWP) 34 times stronger than carbon dioxide (CO2) over a 100-year time period and 96 times stronger over a 20-year time period (Gasser et al, 2017)

  • Natural wetland CH4 emission in Arctic regions is of much interest to the scientific community because the CH4 emissions can potentially increase in a warming climate (AMAP, 2015)

  • We present the first study to analyze the atmospheric CH4 mixing ratios from the above new Environment and Climate Change Canada (ECCC) observational sites located in the Canadian Arctic region

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Summary

Introduction

Atmospheric methane (CH4) is one of the principal greenhouse gases with a global warming potential (GWP) 34 times stronger than carbon dioxide (CO2) over a 100-year time period and 96 times stronger over a 20-year time period (Gasser et al, 2017). Estimated CH4 emissions for the Canadian Arctic (representing the land region of Canada north of 60◦ N) show discrepancies among the inverse studies; the mean annual total CH4 emission (2006– 2010) is ∼ 1.8 Tg CH4 by TM5-4DVAR (Bergamaschi et al, 2013), 0.5 Tg CH4 by CarbonTracker-CH4 (Bruhwiler et al, 2014), and 2.1 Tg CH4 by FLEXINVERT (Thompson et al, 2017). Environment and Climate Change Canada (ECCC) has recently added five greenhouse gas (GHG) measurement sites in northern Canada to monitor the time evolution of Arctic GHGs in view of better constraining flux estimates in the region. We present the first study to analyze the atmospheric CH4 mixing ratios from the above new ECCC observational sites located in the Canadian Arctic region.

Measurements
Site descriptions
Temporal variations
Seasonal and inter-annual variations
Synoptic and diurnal variability
Regional inversion model description
Transport models and meteorological data
LPDM:WRF-STILT
Global background model
Prior fluxes
Wetland CH4 fluxes
Forest fire CH4 fluxes
Anthropogenic emission
Other natural CH4 fluxes
Regional inversion
Atmospheric measurements
Comparison of footprints
Comparison of prior and posterior fluxes with different transport models
Comparison with previous estimates
Relationship of fluxes with climate anomalies
Comparison of modelled and observed mixing ratios
Prior fluxes: wetland CH4 fluxes
Contributions of background CH4 mixing ratios on the posterior fluxes
Conclusions
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