Abstract
Oxoferryl gymnastics: The oxo and CH3CN ligands in 1-NCCH3 can swap positions in the presence of iodosobenzene and tetrafluoroborate anion leading to the generation of a more reactive isomer 2. This conversion is proposed to take place via an activated FeIV unit (1 a) or a transient dioxoiron(VI) species (1 b).
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