Abstract

Persistent Organic Pollutants (POPs) are toxic and difficult to degrade, which will cause huge damages to human life and the ecological environment. Therefore, based on historical measurements, it is important to use intelligent methods and data analysis technologies to build an intelligent prediction system to accurately predict the future POPs concentrations in advance. This work has extremely important significance for policy formulation, human health, environmental protection and the sustainable development of society. Since the POPs concentrations sequence contains both linear and nonlinear components, this paper proposes an intelligent data analysis system combining autoregressive integrated moving average (ARIMA) and long short-term memory network (LSTM) to analyze and predict the POPs concentrations in the Great Lakes region. ARIMA is used to capture linear components while LSTM is used to process nonlinear components, which overcomes the deficiency of single models. Moreover, a one-class SVM algorithm is used to detect outliers during data preprocessing. Bayesian information criterion and grid search methods are also used to obtain the optimal parameter combinations of ARIMA and LSTM, respectively. This paper compares our intelligent data analysis system with other single baseline models by using multiple evaluation indicators and finds that our system has the smallest MAE, RMSE and SMAPE values on all datasets. Meanwhile, our system can predict the trends of concentration changes well and the predicted values are closer to true values, which prove that it can effectively improve the precision of prediction. Finally, our system is used to predict concentration values of sites in the Great Lakes region in the next 5 years. The predicted concentrations present a large fluctuation trend in each year, but the overall trend is downward.

Highlights

  • Introduction published maps and institutional affilPersistent organic pollutants (POPs) are natural or artificially synthesized, difficult to degrade, toxic, bio-accumulative, and can migrate long distances in the atmospheric environment and deposit in remote polar regions of the earth, which is critically harmful to human health and the ecological environment

  • This paper proposes to build an intelligent data analysis system combining autoregressive integrated moving average (ARIMA) and long short-term memory network (LSTM) to intelligently analyze and predict the POPs concentration values in the Great Lakes

  • This paper focuses on the total concentrations sequence of polychlorinated biphenyls (PCBs) in the vapor phase of Electronics 2022, 11, 652 these three monitoring sites

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Summary

Related Work

Data analysis [17] is driven by data, adopting specific methods to summarize, understand and digest the acquired data, so as to develop data functions to a greater extent and utilize the value of data. POPs pose a great threat to human beings and ecological environment, and they have always been the focus of research by environmental scientists from all over the world They want to identify the sources of POPs in a certain area and understand its concentrations change trend like halving times and spatial distribution. PDMS-air partition coefficient, which can help researches better understand the distribution behavior of POPs. Das et al [33] predicted the condition of specific area with a probabilistic approach based on fuzzy Bayesian network, which took consideration of spatial-temporal relationships between climate factors. With the development of deep learning technologies, neural network-based methods are introduced into time series forecasting, which are powerful tools to model nonlinear relationships between sequences. Liang et al [46] applied multi-level attention mechanism in the

Our Proposed Intelligent System
Baseline Models
Our Proposed Intelligent System Combining ARIMA and LSTM
Datasets
Data Preprocessing
Parameter
Parameter Setting for ARIMA
Parameter Setting for RNN and LSTM
Parameter Setting for Our System
Performance Analysis
Evaluation Metrics
Chicago Result
Result
Point Petre Result
Future Prediction
Eagle Harbor Prediction Result
Point Petre Prediction Result
Conclusions and Future
Full Text
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