Abstract
In this Letter the LCAC–SW method has been extended to study the reaction dynamics for ion-pair formation processes on an M+X 2→M ++X 2 − reaction system involving two potential energy surfaces, i.e., the covalence state (M+X 2) and the ionic state (M ++X 2 −), and their crossing effect. The working equations for calculating the state-to-state probability have been derived based on the above two-state model, and the collinear state-selected probabilities for M+I 2→M ++I 2 − (M=Na, K, Cs) ion-pair formation systems have been obtained.
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