Abstract
Abstract In the ESR spectra of N,N-bis(phenylthio)-, N,N-bis(phenyl-d5-thio)-, and N,N-bis(3,5-dichlorophenylthio)aminyls, 33S hyperfine splittings were detected. The spin densities in the aminyls were calculated by using the HMO calculations with and without McLachlan’s correction, and the results were compared with the values derived from the 1H, 14N, and 33S hyperfine splittings by use of the relationship a=Qρ.
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