Abstract
In order to generate powerful radicals as oxidizing species for the complete oxidation of NO, homogeneous activation of peroxymonosulfate (Oxone: PMS) by the Mn3O4/GO catalysts was explored. The catalytic oxidation of NO from waste gas was investigated using advanced oxidation process based on sulfate radicals that produced. The manganese oxide immobilized on graphene oxide (GO) can activate PMS for the oxidation of NO in water. We not only took advantage of the high oxidation–reduction potential of produced sulfite radicals but also an opportunity to oxidize NO on less complex compounds with low dosages. The Mn3O4/GO catalysis system was characterized using X-ray diffraction (XRD) and scanning electron microscopy (SEM). The results showed that Mn3O4was well-distributed on GO. The Mn3O4/GO catalyst system exhibited high efficiency for NO oxidation when the Mn3O4/GO catalyst has an optimum Mn3O4loading. In addition, the best catalytic oxidation can be achieved within 30 min with pH 4 and 6 mM PMS at 25 °C. Therefore, the results indicate promising potential for a system utilizing Mn3O4/PMS to oxidize NO for offgas treatment.
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