Abstract

The relative impact of non-exhaust sources (i.e. road dust, tire wear, road wear and brake wear particles) on urban air quality is increasing. Among them, road dust resuspension has generally the highest impact on PM concentrations but its spatio-temporal variability has been rarely studied and modeled. Some recent studies attempted to observe and describe the time-variability but, as it is driven by traffic and meteorology, uncertainty remains on the seasonality of emissions. The knowledge gap on spatial variability is much wider, as several factors have been pointed out as responsible for road dust build-up: pavement characteristics, traffic intensity and speed, fleet composition, proximity to traffic lights, but also the presence of external sources. However, no parameterization is available as a function of these variables.We investigated mobile road dust smaller than 10 μm (MF10) in two cities with different climatic and traffic conditions (Barcelona and Turin), to explore MF10 seasonal variability and the relationship between MF10 and site characteristics (pavement macrotexture, traffic intensity and proximity to braking zone). Moreover, we provide the first estimates of emission factors in the Po Valley both in summer and winter conditions. Our results showed a good inverse relationship between MF10 and macro-texture, traffic intensity and distance from the nearest braking zone. We also found a clear seasonal effect of road dust emissions, with higher emission in summer, likely due to the lower pavement moisture. These results allowed building a simple empirical mode, predicting maximal dust loadings and, consequently, emission potential, based on the aforementioned data. This model will need to be scaled for meteorological effect, using methods accounting for weather and pavement moisture. This can significantly improve bottom-up emission inventory for spatial allocation of emissions and air quality management, to select those roads with higher emissions for mitigation measures.

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