Abstract

Tracer transport in the atmosphere is controlled not only by synoptic-scale to mesoscale weather disturbances but also by microscale boundary-layer processes especially under fair-weather conditions. The present study investigates numerically the diurnal variation of boundary-layer convection and cumulus clouds and their role in transporting tracers by conducting high-resolution simulations that explicitly resolve turbulent eddies. The transport of dust aerosols in a desert area under two distinct stability conditions is specifically examined. Convection plays a significant role in transporting dust upward; in other words, the vertical depth of the dust transport is critically determined by the depth of convection. Deep convection is effective in transporting dust into the free atmosphere. The early morning stratification strongly regulates the temporal evolution and the vertical growth of convection and therefore the amount of tracer emission and transport. A sensitivity to model resolution of O (1 km) in a cloud-resolving simulation range is also examined. A proper parameterization for activating microscale convection is required for representing the diurnal variation of convection and tracer transport.

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