Abstract
Emissions from biogenic sources are the primary source of isoprene and monoterpene that contribute to the formation of ozone and secondary organic aerosol (SOA). In this study, we used a regional air quality model to examine the sensitivity of simulated ozone to biogenic emission estimates. We created a new regional database of plant functional type (PFT) and land use and land cover (LULC) based on two satellite data products, the Alberta Vegetation Inventory (AVI) and Earth Observation for Sustainable Development of forests (EOSD).The Model for Emissions for Gases and Aerosols from Nature (MEGAN) biogenic emissions model was used with the new PFT data as well as the default Moderate Resolution Imaging Spectroradiometer (MODIS) PFT to generate biogenic emissions in Alberta. The comparison revealed that the new LULC increased isoprene (ISOP) emissions by 30–40 %, decreased monoterpene emissions by 7–8 %, and increased NO emissions by 65–90 % associated with the new regional plant functional type fractional (PFTf) database. This study further investigated the impact of using Alberta-specific biogenic emission on ambient ozone concentration through the Community Multi-scale Air Quality (CMAQ) modeling system against the default MEGAN emissions. In addition, the result from using the new LULC on the predicted fourth highest daily maximum 8-h ozone concentration were examined, which showed a substantial reduction (6 ppb) in ozone in the urbanized capital region area when compared to the default the LULC with less ozone changes in the rural areas. This is likely due to ozone formation in the urban areas being more sensitive to changes in volatile organic compound (VOC) emissions than the rural areas. As CMAQ tended to overestimate the observed ozone peaks in the urban areas, the use of the enhanced LULC resulted in improved model performance compared to the default LULC database. This study results will be primarily used to understand impact of biogenic emission into air on ambient air quality and secondary to provide strategic advice on air quality management plan and initiatives regarding air issues (e.g., ozone) in the region. Results also can be implied to the relationship between climate change-induced increases in biogenic VOC emissions and ozone concentrations.
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