Abstract
Medical X-ray computed tomography requires fast imaging at a low dose rate and in a large area. Halide perovskites have shown high potential for X-ray detection, but a pressing challenge is the current lack of low-cost methods for large-scale fabrication of high-quality thick perovskite films. Here we demonstrate and elucidate an aerosol-liquid-solid process to enable continuous growth of uniform halide perovskites films at low temperature over a large area of 100 cm2, which are vertically monolithic and monocrystalline, and thus beneficial to carrier transport. Direct conversion X-ray detectors based on the representative CsPbI2Br films in conjunction with a deliberated, interface-engineered C-electrode have realized an unprecedented sensitivity (≥1.48×105 μC Gyair−1cm−2). We have further demonstrated the high-resolution radiographic imaging capability of these films. These results lay the groundwork for large scale application of halide perovskites in radiation detectors.
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