Abstract
An amine phase-transfer approach is a novel design for the facile and recyclable fixation and nonbiological mineralization of CO2 into alkaline earth carbonate (MCO3, M = Ca, Sr, and Ba) crystals with uniformed polymorphs at room temperature under atmospheric pressure. The amines’ system based on two phases of water and Zn-tetraphenylporphyrin (ZnTPP) in CH2Cl2 provides a green and sustainable CO2 capture and utilization (CCU) strategy for the mitigation of anthropogenic CO2 emission to the atmosphere.
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