Alignment sensitivity of molecular-frame photoelectron momentum and angular distribution of by XUV attosecond pulses

Abstract

In this work, we investigate the molecular-frame photoelectron momentum and angular distributions (MF-PMD and MF-PAD) of in the presence of XUV Attosecond Pulses. We present the alignment-sensitive effect of MF-PMDs and MF-PADs when the laser field polarization and the molecular axis are close to parallel geometry. Our results show that the MF-PADs and MF-PMDs of single-photon ionization of ion vary drastically when the alignment slightly shifts from parallel geometry to a small alignment angle (e.g. 4°) between the laser polarization direction and the molecular axis at the equilibrium inter-nuclear distance of R c = 2 atomic units. As R c increases to 4 atomic units, such sensitivity is decreased. The R c -dependent transition cross-sections in different channels are found to be the origin of such sensitivity.