Alignment-free difference frequency light source tunable from 5 to 20 µm by mixing two independently tunable OPOs.

Abstract

Tunable mid-infrared ultrashort lasers have become an essential tool in vibrational spectroscopy in recent years. They enabled and pushed a variety of spectroscopic applications due to their high brilliance, beam quality, low noise, and accessible wavelength range up to 20 µm. Many state-of-the-art devices apply difference frequency generation (DFG) to reach the mid-infrared spectral region. Here, birefringent phase-matching is typically employed, resulting in a significant crystal rotation during wavelength tuning. This causes a beam offset, which needs to be compensated to maintain stable beam pointing. This is crucial for any application. In this work, we present a DFG concept, which avoids crystal rotation and eliminates beam pointing variations over a broad wavelength range. It is based on two independently tunable input beams, provided by synchronously pumped parametric seeding units. We compare our concept to the more common DFG approach of mixing the signal and idler beams from a single optical parametric amplifier (OPA) or oscillator (OPO). In comparison, our concept enhances the photon efficiency of wavelengths exceeding 11 µm more than a factor of 10 and we still achieve milliwatts of output power up to 20 µm. This concept enhances DFG setups for beam-pointing-sensitive spectroscopic applications and can enable research at the border between the mid- and far-IR range due to its highly efficient performance.