Air pollution characteristics associated with mesoscale atmospheric patterns in northwest continental Europe

Abstract

An impact related daily air quality index (DAQx), calculated for 15 air quality monitoring stations (traffic, background, and industry) in Belgium, France, Germany and Luxembourg, was compared to mesoscale atmospheric patterns between 2001 and 2007. Meteorological conditions were described by the Hess and Brezowsky synoptic weather classification system and gridded data of the EU FP6 ENSEMBLES project of total precipitation and mean surface temperature. DAQx values indicate sufficient to poor air quality in the urban area of Brussels and at urban traffic stations, as well as satisfactory air quality at the background stations. The air quality index refers to more than 90% to the presence of high PM10, O3 and NO2 concentrations. SO2 and CO play only a minor role. The investigation of weather regimes indicates that zonal and mixed cyclonic circulation regimes are associated with better air quality than meridional and anticyclonic weather regimes. In general, weather regimes with high daily precipitation lead to better air quality than dryer air masses because of lower contribution of PM10 to the air quality index. A trend analysis of weather regimes from 1978 to 2007 shows significant (α = 0.05) positive trends for weather classes associated with lower PM10 concentrations. The results of a case study at a German station examining the relationship between PM10 concentrations and local meteorological quantities (wind speed and precipitation) confirm the results of the regional analysis.