Abstract

We have conducted a time-resolved, two-dimensional light scattering study of the nonlinear dynamics of field-induced structures in an electrorheological fluid subjected to oscillatory shear. We have developed a theoretical description of the observed dynamics by considering the response of a fragmenting and aggregating particle chain to the prevailing hydrodynamic and electrostatic forces. This structural theory is then used to describe the nonlinear rheology of electrorheological fluids.

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