Aerosol effects on liquid cloud microphysical properties in south China: Land–ocean contrasts

Abstract

The aerosol effects on liquid cloud microphysical properties over South China and adjacent ocean regions are investigated by using aerosol reanalysis data from MERRA-2, cloud property data from CLARA-A2, and reanalysis data from ERA5 from 1995 to 2015. The aerosol optical depth (AOD) in South China and adjacent ocean regions shows an upward trend with obvious land–ocean contrasts. The AOD is significantly positively correlated with the liquid cloud droplet effective radius (LREF) over both land and the ocean in summer and autumn, while increasing AOD significantly suppresses the LREF in spring and winter over land. This indicates that the thermal supply is likely the reason for the differences in aerosol effects on liquid cloud properties in different seasons. The weak correlation between the AOD and LREF over the ocean in spring may be because the South China Sea monsoon onset increases the atmospheric instability, and springtime in southeastern China is characterized by high rainfall. This indicates that the effects of aerosols on clouds are not as significant as those on large-scale systems. Further analysis shows that the aerosol effects on the liquid cloud properties are strong and positive at low liquid water paths (LWP) in summer and autumn, while the effect is weak at high LWPs. This may be due to the presence of sufficient liquid water droplets with large LWPs in summer and autumn, and few liquid water droplets in spring and winter. The aerosol effects on liquid cloud properties also significantly depend on lower-tropospheric stability (LTS).