Abstract
The review provides a summary of the current methods of tracing photoexcitation processes and structural dynamics in the solid state, putting major emphasis on the X-ray diffraction techniques (time-resolved Laue diffraction on synchrotron sources and time-resolved serial femtosecond crystallography on X-ray free-electron lasers). The recent developments and nowadays experimental possibilities in the field are discussed along with the data processing and analysis approaches, and illustrated with some striking literature examples of the respective successful studies. Selected complementary methods, such as ultrafast electron diffraction or time-resolved X-ray absorption spectroscopy, are briefly presented.
Highlights
The complexity of real-world systems and their transformations makes theoretical predictions often inaccurate or even not feasible
In the static approach the crystal sample is exposed to a continuous light source (e.g., Xe lamp or light-emitting diode) for a given period of time, after which it is examined using the X-ray diffraction technique
Another solution, microfluid the obtained flow rates amount to min tor), generates thin liquid stream by the action of electric field. Both liquid and vicio electrokinetic sample holder (MESH; known as the electrospin injector), generates matrices can be applied in this method as long as they are sufficiently polarizable in or thin liquid stream by the action of electric field. Both liquid and vicious matrices can be toapplied interact with electric field.asItthey should be notedpolarizable that the experiment is performed und in this method as long are sufficiently in order to interact with vacuum, which may result in evaporation of theissample liquid, orvacuum, dehydration electric field
Summary
The complexity of real-world systems and their transformations makes theoretical predictions often inaccurate or even not feasible. X-ray sources, as small molecules are currently feasible almost exclusively at high-intensity X-raysuch sources, synchrotrons [12,15,16] Laue method, applied such as synchrotrons [12,15,16]. 0 ), and the latter exhibiting larger molecular deformation and a rather long lifetime On the whole, this short review is thought to provide a summary of the methods o of 37 tracing excitation processes and structural dynamics in the solid state, indicate some of the recent important results, and constitute a valuable source of information on what has already been conducted in the field, as well as on the current research possibilities. Tracing excitation processes and structural dynamics in the solid indicate some of the recent important results, and constitute a valuable source of information on what has
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