Abstract
Recent interest in sequestration of carbon dioxide (CO2) in gasified coal seam (i.e., post-underground coal gasification sites) has created a need to understand the coal properties, specifically, the adsorption behavior of CO2 on gasified coal. In the present study, the CO2 excess adsorption isotherms were determined for four coal samples of different characteristics based on the volumetric method. Further, coal chars from a coking coal and a non-coking coal (within the studied samples) were investigated for their CO2 adsorption capacity. The coal samples of size 22–32 mm were pyrolyzed in a drop-tube furnace at 800 and 1000 °C with a heating rate of approximately 2.5 °C s–1 under an inert atmosphere. Measurements were performed up to a pressure of 65 bar for all of the studied samples. Experiments were carried out at an isothermal temperature of 45.5 °C. The influence of coal properties on adsorption was also studied and compared to the literature data. Behavior of adsorption capacities was analyzed as a...
Published Version
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