Abstract

Active nanophotonic materials that can emulate and adapt between many different spectral profiles—with high fidelity and over a broad bandwidth—could have a far-reaching impact, but are challenging to design due to a high-dimensional and complex design space. Here, we show that a metamaterial network of coupled 2D-material nanoresonators in graphene can adaptively match multiple complex absorption spectra via a set of input voltages. To design such networks, we develop a semi-analytical auto-differentiable dipole-coupled model that allows scalable optimization of high-dimensional networks with many elements and voltage signals. As a demonstration of multi-spectral capability, we design a single network capable of mimicking four spectral targets resembling select gases (nitric oxide, nitrogen dioxide, methane, nitrous oxide) with very high fidelity ( >90% ). Our results could impact the design of highly reconfigurable optical materials and platforms for applications in sensing, communication and display technology, and signature and thermal management.

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