Abstract
CH(X 2R) was produced by multiple infrared photon dissociation of CH3OH in the presence of excess atomic oxygen or nitrogen. Time-resolved measurements of relative CH concentrations were made at 298 K with a tunable dye laser. Rate constants deduced from the dependence of CH decay rate on atom concentration are (9.5±1.4)×10−11 cm3 s−1 for CH+O and (2.1±.5)×10−11 cm3 s−1 for CH+N.
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