Abstract

Layered ferromagnetic (FM) materials are significant for nano-spintronic devices, however, low transition temperature and air instability remain major challenges for layered FM compounds. Herein, we have synthesized layered crystals CrIr2Sn10 with FM transition below 315 K. The ratio of the magnetization between in-plane and out-of-plane is 41. Moreover, the magnetism of CrIr2Sn10 is derived from the highly spin-polarized Cr atoms. CrIr2Sn10 will be a promising platform for 2D magnetism and spintronic devices.

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