Abstract
The low-lying intravalence and Rydberg excited states of cyclohepta-1,3,5-triene and cycloocta-1,3,5,7-tetraene, accessed by one- and two-photon absorption, have been investigated at ab initio level by utilizing RPA vertical transition energies and amplitudes. The nature of the first valence-like excited states of cyclohepta-1,3,5-triene has also been studied by CI-SD calculations.
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