Abstract

In recent years, with the widespread application of stretchable electronic devices, the demand for high performance wearable strain sensors is increasing. We propose a simple strategy to prepare a stretchable composite conductor based on the good miscibility of polydimethylsiloxane (PDMS) and poly (3,4-ethylenedioxythiophene):poly (styrenesulfonate) (PEDOT:PSS) under doping. Although the addition of high concentration PEDOT:PSS can improve conductivity, it also reduces the mechanical properties and transmittance of the conductor. The composite conductor containing 20 wt% PEDOT:PSS not only exhibit good electrical conductivity, recovery and piezoresistive effects, but also have excellent tensile properties, transparency and cycle stability. As a core application, composite conductor can be directly attached to human skin as strain sensors for real-time monitoring of the knuckles, elbows and knee joints. In addition, we also reveal the scalability of the conductor preparation technology, that is, the PEDOT:PSS/PDMS blends exhibits satisfactory screen printing suitability. The printed conductor maintains the electrical conductivity and flexibility of the material itself, and the printing effect has no obvious detail missing.

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