Abstract
An nth order truncation of the continued fraction representation of the molecular dipole moment correlation function is introduced from the free rotation representation and an interaction process which is supposed to be governed by a Poisson distribution. We can then derive a general expression for the correlation function, related both to the natural distribution of angular velocities and the successive time derivatives of the mean square torque due to molecular interactions. Some numerical results and comparisons with experiments are given in the second order truncation case.
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