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Abstract
In this paper a theory of chemical reactions is developed which combines stochastic theory and the Franck–Condon transition model. The theory assumes that collision complexes are formed and broken up in a manner similar to the Franck–Condon transition and the collision complexes evolve in time according to the Fokker–Planck equation derived previously for inelastic scattering. The model can be shown to include the RRKM theory as a special case. An illustrative calculation is performed with the example of the H+Cl2 reaction. The result is in qualitative agreement with the result by a numerical solution method.
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