A solid-liquid mixing reactor based on swirling flow technology

Abstract

Solid-liquid mixing is often applied in the chemical industry to keep solids in suspension for, amongst others, crystallization, adsorption, heterogeneous catalysis, etc. The most widely used technology to obtain a good degree of mixing is the mechanically stirred tank reactor. However, this technology is limited to small reactor volumes in case of high pressure/temperature processes due to sealing issues. An alternative for solid-liquid mixing is the application of swirling flow. This work studies the mixing capacities of a specially designed reactor geometry, the Swirling Flow Reactor (SFR). Computational Fluid Dynamics (CFD) is used to simulate the flow field and particle distribution in the SFR, where the RNG k−ϵ model and the Eulerian-Eulerian (E-E) multi-phase approach with a Kinetic Theory of Granular Flow (KTGF) model are applied for their proven effectiveness in the study of dense solid-liquid mixing problems. The effectiveness of mixing in the SFR is assessed by the axial particle distribution and homogeneity H. The mechanism of particle recirculation in the SFR is also identified, in which a Coanda jet flow (CoJF) formed by a specially designed inlet nozzle plays an important role in washing the reactor bottom surface. Additionally, Spectral Proper Orthogonal Decomposition (SPOD) is used to identify and reconstruct the coherent structures in the swirling flow. The results indicate that precessing coherent flow structures are present, which include the dominant double layer double helical vortex core and its second order harmonic, the double layer quadruple helical vortex core.