A SAR protocol for heat-sensitive materials exhibiting sensitization (SARHS) for the estimation of the equivalent dose

Abstract

Accurate estimation of the radiation released at incidents, such as nuclear accidents or radiological terrorist events is of major importance for the prediction of health effects following such an incident. The luminescence properties of several materials are studied in order to assess their potential use as dosimeters in such cases.However, the protocols followed for such purposes are mainly those initially developed for dating. Multiple-aliquot protocols are mainly based on the Thermoluminescence response of the dosimeter used and require the availability of abundant material, while homogeneity of the luminescent substance in the entire sample is also a prerequisite in order to prepare similar aliquots. To account for the above drawbacks, several single-aliquot protocols have been suggested based on Optically Stimulated Luminescence (OSL), which however involve steps of heating the sample up to 300 °C, and as a result they can only be used for heat-resistant materials.In the present work, a novel single aliquot regenerative-dose protocol suitable for heat-sensitive materials exhibiting sensitization (called SARHS) for the estimation of the equivalent dose with OSL is proposed. The protocol eliminates any sensitization effects without encompassing any heating of the sample. Validation of the SARHS protocol was accomplished with three different heat-sensitive materials which exhibit sensitivity changes with the repeated use of the same sample (sensitization), i.e., dragonfly wings, a commercial solid drug (Daktarin) and chicken bones, in which the natural equivalent dose could be successfully recovered with negligible error even when fading, after exposure to irradiation, of the natural OSL signal was taken into account.