A review of the pollution signatures of polycyclic aromatic hydrocarbons in the sediments of the East China Sea

Abstract

Marine sediments serve as crucial reservoirs for polycyclic aromatic hydrocarbons (PAHs), and their PAH signatures offer valuable historical pollution records. This article provides a comprehensive review of the pollution status of 16 priority PAHs in more than 1000 sediments from the East China Sea (ECS). It focuses on the PAH sources, spatiotemporal distributions, driving factors, and ecological risks, with information derived from peer-reviewed papers published between 2003 and 2023. The results revealed that vehicular emissions, mixed combustion sources of coal, biomass, and coke, as well as petrogenic sources, were the primary contributors to PAH pollution in the ECS sediments, accounting for 50%, 34%, and 16%, respectively. Human activities, hydrodynamic mechanisms, and environmental variables such as particle size and organic matter, collectively influenced the distribution of PAHs. Additionally, the population size and economic development played a key role in the temporal distribution of PAHs in the ECS sediments. The ecotoxicity assessment of PAHs in sediments indicated a low risk level. These outcomes are expected to provide environmentalists with detailed and up-to-date insights into sedimentary PAHs in the ECS, helping to develop suitable monitoring plans and strategies for promoting better management of ECS environment.