A reassessment of Nd-isotopes and clay minerals as tracers of the Holocene Pacific water flux through Bering Strait

Abstract

The flux of low-salinity Pacific water (PW) through Bering Strait (BS) weights on the freshwater budget of the Arctic Ocean, which, in turn, impacts the Atlantic Meridional Overturning Circulation (AMOC). Through time, this PW flux has been tightly controlled by the bathymetry of the Strait (~50 m water depth at present), thus by sea-level (SL) changes, as documented in several papers based on a large array of sedimentological and geochemical tracers. The present study aimed at reassessing the robustness of these tracers of the PW-flux, based on five surface samples collected along a south–north transect from BS to the Chukchi Plateau, within the bathymetric range of the PW-mass dispersal. We also estimated their variation in relation to the post-glacial SL-rise in a sedimentary core (ARC4-R09), from the Chukchi shelf, spanning the last ~10 cal kyr. Potential indicators of PW-flux include sortable silt, clay minerals, and the particulate and exchangeable Nd-isotope composition of specific grain-size fractions. The results indicate that ɛNd-values in leachates, and to a lesser extent, the smectite abundance, both relating to volcanic rocks of the Bering Sea, are sensitive indicators of the PW-flux, whereas sortable silts and other clay minerals relative abundances are also influenced by other processes (e.g., west–east shelf currents, sea-ice rafting). The modern distributions of ɛNd-value and smectite abundance illustrate mixing between two endmembers: i) a northern Bering Sea endmember, characterized by ~14% of smectite (vs all clay minerals) and a ɛNd-value of the exchangeable fraction of ~ −2; ii) a Chukchi Sea endmember, characterized by ~8% of smectite and a ɛNd-value ranging from −7 to −8. The Holocene sedimentary record from the study core indicates a progressive increase in Bering Sea supplies through time, linked to an enhanced inflow of PW, which we associate with the deepening of the Strait due to the rising SL. Following a major reorganization of the Arctic Ocean circulation at ~8 cal kyr BP, a steady increase in PW flux prevailed until ~4 cal kyr BP. A tenuous but continuous positive trend towards modern εNd values followed during the late Holocene. The middle Holocene steep increase of warm, low salinity PW-flux through BS, led to important changes in the Arctic Ocean, in particular of its salinity budget. Assuming that the BS bathymetry is the main parameter governing the PW-flux towards the Arctic Ocean, a first-order estimate of PW-flux under a higher than modern SL can be made using the SL-elevation-ɛNd relationship of the major middle Holocene shift.