Abstract
The synthesis of NH3 heavily relies on the Haber-Bosch process suffering from a large amount of CO2 emission and energy consumption. Possessing eco-friendly and sustainable characteristics, electrochemical reduction is considered as a promising candidate for artificial N2 fixation under ambient conditions, but efficient electrocatalysts are crucial for the N2 reduction reaction (NRR). In this communication, we report that perovskite La2Ti2O7 nanosheets behave as an efficient NRR electrocatalyst with excellent selectivity under ambient conditions. In 0.1 M HCl, this catalyst achieves a high NH3 yield rate of 25.15 μg h-1 mgcat.-1 with a faradaic efficiency of 4.55% at -0.55 V vs. a reversible hydrogen electrode. Notably, it also shows high electrochemical stability.
Sign-in/Register to access full text options 
Talk to us
Join us for a 30 min session where you can share your feedback and ask us any queries you have
Schedule a callDisclaimer: All third-party content on this website/platform is and will remain the property of their respective owners and is provided on "as is" basis without any warranties, express or implied. Use of third-party content does not indicate any affiliation, sponsorship with or endorsement by them. Any references to third-party content is to identify the corresponding services and shall be considered fair use under The CopyrightLaw.
