A numerical analysis of multi-dimensional iron flame propagation using boundary-layer resolved simulations

Abstract

Iron combustion is emerging as a topic of immediate interest, given the need for the decarbonization of heat and power generation. Opposite to other solid fuels, iron particles burn predominantly in a non-volatile, heterogeneous combustion mode. For iron dust flames, two modes of flame propagation have been observed i.e. the discrete mode, when the heat transfer time scale is larger than the particle burn-time, and the continuous mode, when the heat transfer timescale is smaller than the burn-time of a single particle. The flame speed of such a flame primarily depends on the heat and mass transfer which is characterized by the distance between the particles for a dispersed mixture. Depending on the variation in particle distance and local distribution, planar or curved flames can form and propagate. The characteristics of flame propagation motivate this study and for the first time, three-dimensional particle boundary layer resolved simulations are used to analyse the effect of curvature and variable particle distances on iron–air flame propagation. Simulations are carried out for (1) planar flame propagation with constant particle spacing in the direction of propagation, and (2) curved flame propagation with varying particle spacing in the direction of propagation. The analysis of the flame speed for the planar flame propagation later guides the analysis of curved flames propagating through 900 boundary-layer resolved particles distributed in a 30 by 30 grid. The curved flame propagates with a uniform but decreased flame speed compared to the planar flame propagation with equivalent particle spacing. It is shown that positive curvature decreases the heat transfer from the burnt to the unburnt side while a variable spatial arrangement of particles allows for a local re-distribution of oxygen which causes some regions to burn richer or leaner than the corresponding planar flames with similar particle spacing.