A novel model for the determination of nanoparticle impact velocity in low pressure impactors

Abstract

The crucial parameter in the analysis of impact events is the impact velocity vi. In case of inertial impactors vi was assumed to be 85% of the average gas jet velocity, following the work of Marple. Numerical analysis of the impact process in low pressure impactors shows that this assumption is inappropriate and leads to overestimation of vi near the inset of particle deposition, while vi is underestimated in the regime of high impact velocities. In this paper the whole process of nanoparticle acceleration and impact in low pressure impactors is investigated numerically. In order to assure correct numerical procedures, the employed methods are thoroughly validated by comparison with experimental results. Finally, a new analytical model for the calculation of vi on the basis of similarity theory is proposed that is independent of the impactor geometry and particle properties and holds well for the whole incompressible region. The model allows to perform defined collision experiments in low pressure impactors regarding impact velocity, without need of demanding numerical effort that is often beyond the scope of experimental studies. The model replaces the old rule of thumb and allows a quantitative re-evaluation of existing experimental data, e.g. on nanoparticle agglomerate fragmentation.