Abstract
By using azobenzene-4,4′-dicarboxylate (H2L) ligand, a new coordination polymer, formulated as [Mn(L)(H2O)2]n (1), has been synthesized successfully under solvothermal conditions. Complex 1 exhibits a three-dimensional (3D) framework with (4,4)-connected {65.8} topology. Moreover, the fluorescent property of complex 1 has been investigated. The electrochemical study displays that complex 1 forms a re-organization of energy level due to its single-crystal structure in the tandem structure of complex 1/N719/TiO2. The result demonstrates that the complex 1/N719/TiO2 solar cell exhibited excellent photovoltaic performance with the photoelectric conversion efficiency of 3.70% under 100 mW cm−2 illumination.
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