Abstract

Interfacial solar-driven evaporation technology has great potential to address freshwater shortages. Despite significant progress in developing efficient evaporators, the challenge of evaporation rates of two-dimensional evaporators still needs to be solved. In addition, interfacial solar-driven evaporation relies on solar energy to trigger the evaporation of thin water layers at the water–air interfaces. It thus may be at risk of interruption in the absence of sunlight. To overcome these challenges, we have intelligently assembled different functional components to form a multistage assembled lamellar membrane used for interfacial solar-driven evaporation during the day and power generation at night. Specifically, solar evaporation achieved a high evaporation rate of 1.78 kg m−2h−1 under single solar irradiation. Desalination and water purification capabilities were also demonstrated. More notably, the membrane also showed its worth as an electrical generator in overcast weather or nights, delivering a voltage of 309 mV and a current of 2 μA. The voltage and current can be multiplied by connecting four membranes in series and parallel to 1.1 V and 8.8 μA, respectively. This powers a calculator directly and stores excess electricity in a capacitor, which can be as high as 2 V in 2000 s. This innovation shows promising applications in next-generation freshwater production and power generation.

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