Abstract
ABSTRACT Numerical simulations are used to study effects of ozone (O3) and thermal enhancement on autoignition and subsequent burning characteristics of isolated n-heptane droplets in microgravity conditions. Particular focus is given to effects of O3 on low temperature combustion, or cool flames. Levels of ambient O3 mole fraction and ambient temperature are varied from 0 to 0.03 and 400 K to 750 K, respectively. A comparison between two low temperature chemistry enhancement strategies – O3 addition and temperature increase – are investigated on an equivalent energy addition basis to evaluate relative effects on combustion characteristics. Results of this study are analyzed using physical and mixture fraction approaches because of unique insights offered by these frameworks. Ignition and ensuing flame propagation are investigated via a most reactive mixture analysis, evaluated using homogeneous reactor simulations of mixture compositions and temperatures surrounding the droplet. Lastly, a Damköhler number analysis is performed to explore oscillatory ignition dynamics.
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