Abstract
A new computational procedure and a new transition probability expression have been incorporated into the Bauer, Fisher, and Gilmore (BFG) model for quenching and E—V energy transfer. The new transition probability expression takes into account trajectories that are classically allowed on the lower adiabatic potential energy surface, but are classically forbidden on the diabatic surfaces. The calculated quenching cross section reported are in substantially better agreement with experiment than those calculated according to the original BFG model. Further modifications to the BFG model are proposed that could have major effects on the calculated cross sections.
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